The RNA origin of transfer RNA aminoacylation and beyond

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The RNA origin of transfer RNA aminoacylation and beyond.

Aminoacylation of tRNA is an essential event in the translation system. Although in the modern system protein enzymes play the sole role in tRNA aminoacylation, in the primitive translation system RNA molecules could have catalysed aminoacylation onto tRNA or tRNA-like molecules. Even though such RNA enzymes so far are not identified from known organisms, in vitro selection has generated such R...

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The origin of homochirality of l-amino acids has long been a mystery. Aminoacylation of tRNA might have provided chiral selectivity, since it is the first process encountered by amino acids and RNA. An RNA minihelix (progenitor of the modern tRNA) was aminoacylated by an aminoacyl phosphate oligonucleotide that exhibited a clear preference for l- as opposed to d-amino acids. A mirror-image RNA ...

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Stationary-phase expression and aminoacylation of a transfer-RNA-like small RNA.

Genome-scale analyses have shown numerous functional duplications in the canonical translational machinery. One of the most striking examples is the occurrence of unrelated class I and class II lysyl-transfer RNA synthetases (LysRS), which together may aminoacylate non-canonical tRNAs. We show that, in Bacillus cereus, the two LysRSs together aminoacylate a small RNA of unknown function named t...

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It has been shown that the 2’ endoautoaminoacylation of surface-bound RNA is stereoselective for the Lenantiomers of the amino acids (1). This mimics selection of amino acids by RNA in an early ‘RNA world’ (2), and thus may have led to the evolution of L-amino acid homochirality. However, the current selection of amino acids for protein synthesis utilizes the 3’ exoaminoacylated species exclusi...

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ژورنال

عنوان ژورنال: Philosophical Transactions of the Royal Society B: Biological Sciences

سال: 2011

ISSN: 0962-8436,1471-2970

DOI: 10.1098/rstb.2011.0137